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- Description:
- There is considerable technical interest in the improvement of battery technology, as it would allow for the enhancement and realization of many different applications, including the continued miniaturization of portable computational devices, plug-in electric vehicles, and intermittent power storage. Lithium metal represents a theoretical limit on the anode energy density...
- Keyword:
- battery, SEI, scanning probe, mechanical, and lithium
- Subject:
- Materials Science and Energy
- Creator:
- Campbell, Colin Thomas
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/01/2021
- Date Created:
- 2020-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:15275 and etdadmin_upload_764606
-
- Description:
- Elemental powder blends are an emerging alternative to prealloyed powders for high-throughput alloy design via additive manufacturing techniques due to their flexibility, low cost, and ease of customization. This dissertation investigates elemental alloying elements (Sc and Zr) which are high-melting and highly reactive, unlike previous work which focused on more...
- Keyword:
- additive manufacturing, in situ diffraction, elemental blends, laser powder-bed fusion, aluminum, and creep
- Subject:
- Materials Science
- Creator:
- Glerum, Jennifer Anne
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/16/2023
- Date Created:
- 2022-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:16304 and etdadmin_upload_936163
-
- Description:
- As demonstrated by efforts in graphene commercialization, scalable synthesis and high-quality material availability are primary limiting factors for the realization of technologies based on two-dimensional (2D) materials. Thus, in considering the fate of emergent 2D materials such as the metal chalcogenides, the challenge of scalable synthesis is a highly relevant...
- Keyword:
- 2D Materials, Pulsed Laser Deposition, Applied Sciences, Metal Chalcogenides, and Chemical Vapor Deposition
- Subject:
- Nanotechnology, Nanoscience, and Materials Science
- Creator:
- Bergeron, Hadallia
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/01/2021
- Date Created:
- 2020-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:15165 and etdadmin_upload_750151
-
- Description:
- Nanotechnology research broadly encompasses the exploration of the unique chemical,optical, electronic, or biological properties of materials with dimensions < 1 µm. Inorganic nanoparticles are one such class of materials, with properties that are exceptionally sensitive to particle size and structure. This is especially evident in the field of heterogeneous chemical...
- Keyword:
- Parallelized, Catalysis, Nanoreactor, Nanoparticle, and Synthesis
- Subject:
- Nanotechnology, Materials Science, and Chemical engineering
- Creator:
- Jibril, Liban
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 06/22/2022
- Date Created:
- 2022-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:16023 and etdadmin_upload_899605
-
- Description:
- Soft materials in nature are formed through programmed self-assembly of biomolecules to create complex architectures and optimized physical properties. It is therefore a key challenge in biomaterials science and engineering to understand the principles that govern the structure and properties of such materials, and the interactions between their different components....
- Subject:
- Materials Science and Biomedical engineering
- Creator:
- Sangji, Mohammad Hussain
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 10/07/2021
- Date Created:
- 2020-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_816157 and http://dissertations.umi.com/northwestern:15536
-
- Description:
- Transport along and across the grain boundaries of solid-state electrolytes has implications for a broad range of materials and in an equally broad range of technologies. Over the past 2-3 decades, a substantial body of literature has been developed to explain grain boundary transport properties within the context of space...
- Keyword:
- Grain Boundary Charge Transport, Oxide Electrolytes, Electron Holography, Impedance Spectroscopy, Atom Probe Tomography, and Space Charge Theory
- Subject:
- Applied physics and Materials Science
- Creator:
- Xu, Xin
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2019-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14848 and etdadmin_upload_686556
-
- Description:
- Nanoparticle synthesis is capable of producing particles with any combination of structure, chemistry, size, shape, and surface. All of the different combinations of these physical properties can produce nanoparticles with almost countless materials properties suited for many applications. Given this interest in using nanoparticles in so many different fields, including...
- Keyword:
- nanoparticle growth, thermodynamics, nanoparticles, kinetics, hydrothermal synthesis, and crystal growth
- Subject:
- Inorganic chemistry, Chemistry, and Materials Science
- Creator:
- Ly, Tiffany
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 10/07/2021
- Date Created:
- 2021-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:15645 and etdadmin_upload_832870
-
- Description:
- In the late 2000’s, scientific studies in cultural heritage saw a great advancement in macro X-ray fluorescence (XRF) imaging of paintings. These images are used to generate elemental distribution maps, which aid in identifying chemical elements and paint pig- ments as well as their locations throughout the layers of the...
- Keyword:
- machine learning, x-ray fluorescence, and image processing
- Subject:
- Artificial intelligence, Materials Science, and Computer science
- Creator:
- Chopp, Henry Hayashi
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 08/23/2023
- Date Created:
- 2023-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_998414 and http://dissertations.umi.com/northwestern:16642
-
- Description:
- One of the central challenges in solid-state chemistry is synthetic control over structure. Owing to limited reactivity of Pb with transition metals at ambient pressure and high temperature as well as the variety of properties that emerge from the few known binary transition-metal–Pb compounds, this research focuses on accessing and...
- Subject:
- Chemistry and Materials Science
- Creator:
- Tamerius, Alexandra
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 10/07/2021
- Date Created:
- 2021-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_845128 and http://dissertations.umi.com/northwestern:15755
-
- Description:
- Materials science has been central to human advancement since time immemorial. There has always been curiosity around studying the processes required to extract materials, examine their structure, and ultimately tailor their properties to meet human needs. Over the last few centuries, the ability to tailor material properties was driven by...
- Keyword:
- Gaussian Process, Mixed Variable Machine Learning, Data Centric Design, Multicriteria Optimization, and Microstructure
- Subject:
- Materials Science, Statistics, and Design
- Creator:
- Iyer, Akshay
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/02/2022
- Date Created:
- 2021-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_851800 and http://dissertations.umi.com/northwestern:15801
-
- Description:
- This dissertation explores the fundamental science of flexoelectricity and its implications using a combined experimental and theoretical approach. I begin by introducing the flexoelectric effect and formalizing the basics of strain gradients, polarization, and flexoelectric coefficients. Next, I describe the development of a flexoelectric characterization system based upon three-point bending...
- Keyword:
- Oxides, First Principles, Triboelectricity, Flexoelectricity, and Surfaces
- Subject:
- Physics and Materials Science
- Creator:
- Mizzi, Christopher Adam
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 06/28/2021
- Date Created:
- 2021-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:15527 and etdadmin_upload_815247
-
- Description:
- Polymer and polymer/ceramic composites known as bone cements are commonly used in musculoskeletal reconstructive surgeries where bone tissue fixation, reinforcement, or void filling may be needed. Polymethylmethacrylate, PMMA, was the initial (and currently only) FDA-approved bone cement for bone-void filling applications yet faces many inherent material-based challenges that impacts its...
- Keyword:
- Citrate-based biomaterials, V70, Hydroxyapatite, Bone Cement, Vertebral Body Fractures, and Polymethylmethacrylate
- Subject:
- Polymer chemistry, Materials Science, and Biomedical engineering
- Creator:
- Huddleston, Samantha
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 09/22/2022
- Date Created:
- 2022-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:16143 and etdadmin_upload_915696
-
- Description:
- Discrete molecules, linear and branched polymers, and disordered cross-linked networks are well studied objects of chemical synthesis. However, two-dimensional polymers (2DPs) have been long missing from this continuum of molecular architectures, both in chemical synthesis and in Nature. Recently, new polymerization strategies and characterization methods have enabled the unambiguous realization...
- Keyword:
- Covalent Organic Frameworks, Controlled Polymerization, Organic Electronics, and Two-dimensional Polymers
- Subject:
- Polymer chemistry, Chemistry, and Materials Science
- Creator:
- Evans, Austin Michael
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 04/15/2021
- Date Created:
- 2020-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_793170 and http://dissertations.umi.com/northwestern:15454
-
- Description:
- Additive manufacturing is a promising process that has the capability to build components with complex geometries for structural and biomedical applications. Due to the rapid and localized directional solidification of molten metallic alloys, unique phase transformations occur at the melt pool that can provide for components with greater strength and...
- Subject:
- Materials Science and Mechanical engineering
- Creator:
- Wolff, Sarah
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2018-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14448 and etdadmin_upload_626097
-
- Description:
- This thesis describes a series of fundamental studies that address the role of electrostatic interactions in modulating i) the permeability of the ligand shell of a colloidal quantum dot (QD) to an anionic redox probe; ii) the resulting yield of photoinduced electron exchange within the QD ‒ redox probe complex;...
- Keyword:
- electrostatic interactions, surface chemistry, quantum dots, and optical spectroscopy
- Subject:
- Physical chemistry, Nanoscience, and Materials Science
- Creator:
- He, Chen
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2018-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_613994 and http://dissertations.umi.com/northwestern:14389
-
- Description:
- Single-use plastic waste pollution will cause significant harm to the environment if left unaddressed. One possible mitigation strategy is to develop processes, e.g. catalytic hydrogenolysis, that can convert (i.e. upcycle) waste plastics into value-added products capable of participating in a circular economy. Platinum (Pt) catalysts on strontium titanate nanocuboid supports...
- Subject:
- Chemistry and Materials Science
- Creator:
- Peczak, Ian Lukasz
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 05/31/2023
- Date Created:
- 2023-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:16513 and etdadmin_upload_983506
-
- Description:
- Thermoelectric devices convert between temperature gradients and electricity, implying numerous applications, such as powering exploratory space vehicles, industrial waste-heat recovery, and solid- state refrigeration. Thermoelectric devices consist of doped p-type and n-type semiconductor legs, and the overall device efficiency depends on the transport properties of these semiconductor materials. High-performing thermoelectric...
- Keyword:
- band engineering, electronic structure, density functional theory, thermoelectrics, group theory, and tight-binding
- Subject:
- Materials Science
- Creator:
- Brod, Madison K
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 05/31/2023
- Date Created:
- 2023-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:16437 and etdadmin_upload_967109
-
- Description:
- Dilute Al-Sc-Zr-Si-based aluminum alloys retain their strength for long periods of time at elevated temperatures due to a dispersion of nanometric, coherent, and coarsening-resistant Al3(Sc,Zr) (L12 structure) nanoprecipitates that are formed upon aging. These alloys are attractive for replacement of dense steels and costly Ti alloys in the 250–400 °C...
- Keyword:
- L12 nanoprecipitates, Atom-probe tomography, Coarsening, High-temperature alloys, Creep, and Aluminum alloys
- Subject:
- Materials Science
- Creator:
- Michi, Richard Andrew
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 04/29/2020
- Date Created:
- 2020-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_718569 and http://dissertations.umi.com/northwestern:14999
-
- Description:
- Engineering heat transport in materials is essential for thermal management in a wide range of technologies, from batteries to thermoelectrics. Materials host a wide spectrum of heat-carrying phonons, which vary in their frequency, spatial extent, and degree of plane-wave character. This diversity in phonon properties leads to complex behavior, especially...
- Keyword:
- thermal modelling, thermal conductivity, semiconductors, phonons, and thermoelectrics
- Subject:
- Physics and Materials Science
- Creator:
- Gurunathan, Ramya
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/02/2022
- Date Created:
- 2021-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_856415 and http://dissertations.umi.com/northwestern:15824
-
- Description:
- Organic solar cells (OSC) are a next generation solar energy technology that offers the advantages of scalable fabrication, light weight, flexibility, and earth-abundant starting materials. Despite tremendous advances in OSC power conversion efficiency (PCE) over the last decade, active layer material selection and optimization is still largely empirical. In order...
- Keyword:
- Small molecule, Non Fullerene, Crystal Structure, Photovoltaic, and Organic solar Cells
- Subject:
- Chemistry, Materials Science, and Energy
- Creator:
- Swick, Steven Mitomu
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 04/28/2020
- Date Created:
- 2019-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14961 and etdadmin_upload_712474
-
- Description:
- Self-assembly of colloidal particles at the nano- and microscale has been a powerful tool for producing structures with emergent properties in applications ranging from electro-mechanical systems to photonics and biomedical devices. Great success has been achieved in experiments, where a variety of exotic phases have been discovered and even reconfigurable...
- Keyword:
- Soft materials, Computer simulation, Nanoparticles, Self-assembly, and Electrostatics
- Subject:
- Materials Science and Computational physics
- Creator:
- Wang, Ziwei
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/01/2021
- Date Created:
- 2020-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_747162 and http://dissertations.umi.com/northwestern:15154
-
- Description:
- The field of materials discovery is undergoing an unprecedented transition from laboratory tocomputer. Behind this transition is the new ability to accurately compute material properties, especially energetic stability, from first principles with density functional theory (DFT). However, DFT remains computationally expensive, and DFT-based materials discovery is intractable, especially in high...
- Keyword:
- High throughput, Inorganic compounds, Big data, Density functional theory, Materials discovery, and Machine learning
- Subject:
- Materials Science, Condensed matter physics, and Computational chemistry
- Creator:
- Griesemer, Sean Darius
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 05/31/2023
- Date Created:
- 2023-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:16606 and etdadmin_upload_986816
-
- Description:
- Rapid changes in global climate are pushing nations to reduce CO2 emissions and adopt clean energy technologies for renewable energy generation and storage. As wind and solar are implemented worldwide, a commensurate response in energy storage will need to be installed to meet fluctuations in peak energy demands and generation...
- Keyword:
- Fuel cells, Solid Oxide Fuel Cells, SOFC, Solid Oxide Electrolysis Cells, Electrochemistry, and Energy
- Subject:
- Materials Science, Energy, and Engineering
- Creator:
- Lu, Matthew Yunching
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2019-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_685843 and http://dissertations.umi.com/northwestern:14817
-
- Description:
- Water vapor condenses into liquid water when it encounters a cold surface. If the surface temperature is sufficiently low, freezing follows the condensation step, and the process is holistically referred to as condensation frosting. Both phase change processes are fundamental to many industries ranging from water harvesting, thermal management, solar...
- Keyword:
- Frosting, Condensation, Phase Change, Mass Transport, Diffusion, and Droplet
- Subject:
- Applied physics and Materials Science
- Creator:
- Yao, Yuehan
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 04/29/2020
- Date Created:
- 2020-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14997 and etdadmin_upload_718499
-
- Description:
- Recent advances in high-performance computing have resulted in massive databases of materials properties calculated with techniques such as ab initio density functional theory. In fact, some of the largest of such databases have calculations of nearly all distinct, ordered, experimentally-reported compounds. This thesis discusses the application of data in one...
- Keyword:
- high-pressure, OQMD, complex networks, density functional theory, high-throughput, and materials discovery
- Subject:
- Materials Science and Computational physics
- Creator:
- Ishwar Hegde, Vinay
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/01/2021
- Date Created:
- 2019-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_780845 and http://dissertations.umi.com/northwestern:15403
-
- Description:
- Polymers occupied nearly every facet of our daily lives, and enhancing their mechanical and fracture properties has long been an important topic in the field of polymer science. Based on the various need in applications, polymers are designed to have a range of characteristics such as tackiness, optical properties, mechanical...
- Keyword:
- Adhesive, Fatigue, Elastomer, Fracture, Composite, and Mechanical Properties
- Subject:
- Materials Science
- Creator:
- Chen, Qihua
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 08/23/2023
- Date Created:
- 2023-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_1004779 and http://dissertations.umi.com/northwestern:16673
-
- Description:
- Electrochemical cell devices are increasingly being sought for energy conversion and storage applications due to their high efficiencies and their potential for operating free of greenhouse gas (GHG) emissions. Solid Acid Electrochemical Cells (SAECs), which most commonly employ CsH2PO4 (CDP) as the electrolyte component, are uniquely suited to meet the...
- Keyword:
- Cesium Dihydrogen Phosphate, Catalysis, Ammonia, Hydrogen, and Electrochemistry
- Subject:
- Chemistry, Materials Science, and Energy
- Creator:
- Plymill, Austin Blake
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 04/15/2021
- Date Modified:
- 04/15/2021
- Date Created:
- 2021-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_796377 and http://dissertations.umi.com/northwestern:15469
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