Semiconductor nanocrystals possess unique photophysical properties that make them desirable for many optoelectronic applications such as photovoltaics, LEDs, and quantum computing. When the size of a semiconductor is reduced to below the excitonic Bohr radius of the material, its carriers becomes quantum confined resulting in drastic changes to optical, electronic,...
This thesis presents results and analysis on a series of donor-bridge-acceptor (D-B-A) charge transfer systems in which we use time-resolved spectroscopy and magnetic resonance techniques to study the relationship of molecular structure to energy, charge, and spin transfer dynamics. We find that the sequence of events following the initial charge...