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-
- Description:
- Colloidal crystal engineering with DNA offers new opportunities for materials scientists to build and program the structures of superlattices beyond what can be accomplished in Nature with atomic crystal lattices. Thus far, such materials primarily have been studied for their optical properties due to the insulating nature of the DNA...
- Keyword:
- Nanoparticles, Self-Assembly, Surface Modification, and Colloidal Crystal Engineering
- Subject:
- Nanotechnology, Nanoscience, and Materials Science
- Creator:
- Oh, Taegon
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2019-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14533 and etdadmin_upload_640128
-
- Description:
- The heart of computational materials science lies in providing fundamental insights and understanding of materials behavior and properties across different scales. The significance of this task is highlighted by the Materials Genome Initiative and the emergence of computational tools and frameworks such as materials by design, microstructure sensitive design, and...
- Keyword:
- random Process, Multiscale simulation, Microstructure, Gaussian process, and Uncertainty
- Subject:
- Materials Science, Statistics, and Mechanical engineering
- Creator:
- Bostanabad, Ramin
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2019-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14508 and etdadmin_upload_638165
-
- Description:
- Nucleic acids not only are the building blocks of life but also a class of attractive macromolecular therapeutics. However, the delivery of therapeutic oligonucleotides into cells has been a major challenge due to their large size and highly negatively charged backbone. Spherical nucleic acids (SNAs) are a class of emerging...
- Keyword:
- Nanomedicine, Gene regulation, and Drug delivery
- Subject:
- Materials Science, Biomedical engineering, and Chemical engineering
- Creator:
- Zhu, Shengshuang
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2019-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_672179 and http://dissertations.umi.com/northwestern:14728
-
- Description:
- Non-covalent and ion-specific interactions in the context of charged polymers are ubiquitous in nature and in synthetic applications. For example, mussels utilize metal-coordinate bonds to form tough underwater adhesion to a wide range of substrates. The sandcastle worm uses coacervation of oppositely charged polymers to build robust structures for self-defense....
- Keyword:
- Coacervate, Polyelectrolytes, Polymer Mechanics, Quartz Crystal Microbalance, Oil/Water Interface, and Coatings
- Subject:
- Polymer chemistry and Materials Science
- Creator:
- Sadman, Kazi
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2019-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14664 and etdadmin_upload_662829
-
- Description:
- To relate the mechanical responses of hard-soft copolymer systems with their microstructures, a coarse-grained molecular dynamics (CGMD) approach is employed. With the generic bead-spring polymer model mapped from atomistic simulations, this dissertation first studies the morphology of structures with various hard-soft compositions and interactions between hard beads. Following that, this...
- Keyword:
- coarse-grained molecular dynamics, local modulus, polyurea, micro-phase separation, interphase, and viscoelasticity
- Subject:
- Molecular physics, Materials Science, and Mechanical engineering
- Creator:
- Zhang, Min
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2018-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14464 and etdadmin_upload_626984
-
- Description:
- The start of the 21st century brought the sweeping proliferation of portable electronics such as laptops, tablets, and smartphones. These technologies were largely enabled by advances in energy storage methods – lithium ion batteries in particular. Society's push for more advanced energy storage applications, such as electric vehicles, stresses the...
- Keyword:
- conversion reaction, transmission electron microscopy, intercalation electrode, lithium ion battery, and electron energy loss spectroscopy
- Subject:
- Materials Science
- Creator:
- Castro, Fernando Cuauhtli
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2018-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_621102 and http://dissertations.umi.com/northwestern:14419
-
- Description:
- Two-dimensional (2D) materials are a promising class of electronic materials that have generated great interest to improve and create new and existing technologies. The promise of this family of materials relies on their high surface-to-volume ratio and atomic thickness in addition to their unique (opto)electric properties. However, these morphological properties...
- Keyword:
- Two-dimensional, Indium Selenide, Electronics, Black Phosphorus, Passivation, and Liquid phase exfoliation
- Subject:
- Materials Science
- Creator:
- Wells, Spencer Allan
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2018-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_617587 and http://dissertations.umi.com/northwestern:14403
-
- Description:
- In the United States and around the world, the growing energy demands and climate concerns necessitate renewable and efficient energy production. Thermoelectric materials could be one small part of this larger picture movement, but their high cost and low efficiency must be improved to realize commercial use. To decrease the...
- Keyword:
- experimental, semi-empirical model, carrier concentration, dopability, Thermoelectric, and statistical and machine learning
- Subject:
- Materials Science
- Creator:
- Miller, Samuel A
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2018-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_612765 and http://dissertations.umi.com/northwestern:14381
-
- Description:
- Soft materials such as colloids and polymers often exhibit a variety of mesoscopic structures that are governed merely by weak physical interactions. Due to these intermediate structures, they can be easily taken out of thermal equilibrium by introducing external stimuli such as a shear flow and electromagnetic fields. This thesis...
- Keyword:
- Phase transition, Nonequilibrium dynamics, Coarse-grained simulations, Self-assembly, Soft matter, and Machine Learning
- Subject:
- Materials Science, Computational physics, and Statistical physics
- Creator:
- Han, Ming
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2018-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14411 and etdadmin_upload_618073
-
- Description:
- One of the grand challenges in science is development of soft materials that mimic living organisms to optimize the way we use energy, translate or morph reversibly or sense their envi- ronment and respond in a useful fashion. Using the insights from studying biological structures, we hope to design soft...
- Subject:
- Materials Science, Biochemistry, and Computational chemistry
- Creator:
- Iscen, Aysenur
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2019-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14770 and etdadmin_upload_679718
-
- Description:
- Ultrafine particles are often used as lubricant additives because they can enter tribological contacts to reduce friction and protect surfaces from wear. They tend to be more stable than molecular additives under high thermal and mechanical stresses during rubbing. However, in lubricant oil, ultrafine particles tend to aggregate together to...
- Keyword:
- Graphene, Librication, and Tribology
- Subject:
- Materials Science
- Creator:
- Dou, Xuan
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2018-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14400 and etdadmin_upload_616912
-
- Description:
- The halide perovskites AMX3 (A = large cation, B = Sn or Pb, and X = halide) have been the subject of intense investigation due to their outstanding optical and electronic properties, which have enabled high solar cell efficiencies thanks to a beneficial electronic structure and long charge carrier lifetimes....
- Keyword:
- exciton, halide perovskite, semiconductor, radiation detector, and self-trapped exciton
- Subject:
- Inorganic chemistry, Applied physics, and Materials Science
- Creator:
- McCall, Kyle Matthew
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2019-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14511 and etdadmin_upload_638483
-
- Description:
- Rationally assembled nanostructures exhibit distinct physical and chemical properties beyond their individual units. The development of nanofabrication tools enables precise structural defining of nanomaterials scalable to large areas. This dissertation focuses on plasmonic nanoparticle arrays that show unique diffractive coupling with lattice spacings engineered close to the wavelength of light....
- Keyword:
- Light-matter interactions, Metal nanoparticles, Plasmonic superlattices, Upconverting nanolasing, Nanoscale lasers, and Stretchable photonics
- Subject:
- Optics, Nanoscience, and Materials Science
- Creator:
- Wang, Danqing
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2019-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14605 and etdadmin_upload_661446
-
- Description:
- Transport along and across the grain boundaries of solid-state electrolytes has implications for a broad range of materials and in an equally broad range of technologies. Over the past 2-3 decades, a substantial body of literature has been developed to explain grain boundary transport properties within the context of space...
- Keyword:
- Grain Boundary Charge Transport, Oxide Electrolytes, Electron Holography, Impedance Spectroscopy, Atom Probe Tomography, and Space Charge Theory
- Subject:
- Applied physics and Materials Science
- Creator:
- Xu, Xin
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2019-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14848 and etdadmin_upload_686556
-
- Description:
- Additive manufacturing is a promising process that has the capability to build components with complex geometries for structural and biomedical applications. Due to the rapid and localized directional solidification of molten metallic alloys, unique phase transformations occur at the melt pool that can provide for components with greater strength and...
- Subject:
- Materials Science and Mechanical engineering
- Creator:
- Wolff, Sarah
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2018-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14448 and etdadmin_upload_626097
-
- Description:
- This thesis describes a series of fundamental studies that address the role of electrostatic interactions in modulating i) the permeability of the ligand shell of a colloidal quantum dot (QD) to an anionic redox probe; ii) the resulting yield of photoinduced electron exchange within the QD ‒ redox probe complex;...
- Keyword:
- electrostatic interactions, surface chemistry, quantum dots, and optical spectroscopy
- Subject:
- Physical chemistry, Nanoscience, and Materials Science
- Creator:
- He, Chen
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2018-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_613994 and http://dissertations.umi.com/northwestern:14389
-
- Description:
- Rapid changes in global climate are pushing nations to reduce CO2 emissions and adopt clean energy technologies for renewable energy generation and storage. As wind and solar are implemented worldwide, a commensurate response in energy storage will need to be installed to meet fluctuations in peak energy demands and generation...
- Keyword:
- Fuel cells, Solid Oxide Fuel Cells, SOFC, Solid Oxide Electrolysis Cells, Electrochemistry, and Energy
- Subject:
- Materials Science, Energy, and Engineering
- Creator:
- Lu, Matthew Yunching
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 02/12/2020
- Date Created:
- 2019-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- etdadmin_upload_685843 and http://dissertations.umi.com/northwestern:14817
-
- Description:
- Modeling the mechanical performance of metal produced with additive manufacturing (AM) has proven to be a challenging task. In the as-built state, these materials have been shown to exhibit strong heterogeneity and anisotropy. Even after post-processing, such as heat treatment or hot isostatic pressing and depending on the alloy, some...
- Keyword:
- Simulations, Additive manufacturing, Mechanical performance, and Solid mechanics
- Subject:
- Mechanics, Materials Science, and Mechanical engineering
- Creator:
- Kafka, Orion Landauer
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 04/28/2020
- Date Created:
- 2019-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14952 and etdadmin_upload_708678
-
- Description:
- Organic solar cells (OSC) are a next generation solar energy technology that offers the advantages of scalable fabrication, light weight, flexibility, and earth-abundant starting materials. Despite tremendous advances in OSC power conversion efficiency (PCE) over the last decade, active layer material selection and optimization is still largely empirical. In order...
- Keyword:
- Small molecule, Non Fullerene, Crystal Structure, Photovoltaic, and Organic solar Cells
- Subject:
- Chemistry, Materials Science, and Energy
- Creator:
- Swick, Steven Mitomu
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 04/28/2020
- Date Created:
- 2019-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14961 and etdadmin_upload_712474
-
- Description:
- Low-dimensional materials have emerged as a promising platform for ultrathin electronic and optoelectronic devices. The span of electronic properties covers the spectrum from metallic through small and medium bandgap semiconductors to large bandgap insulators, providing all the necessary components to fabricate a variety of devices. Compared to bulk-semiconductor based devices,...
- Keyword:
- Gaussian, self-aligned, spiking neuron, antiambipolar, low-dimensional materials, and van der Waals heterojunction
- Subject:
- Applied physics, Electrical engineering, and Materials Science
- Creator:
- Beck, Megan
- Owner:
- Scholarly Digital Publishing
- Language:
- en
- Date Uploaded:
- 04/29/2020
- Date Created:
- 2020-01-01
- Resource Type:
- Dissertation
- Alternate Identifier:
- http://dissertations.umi.com/northwestern:14986 and etdadmin_upload_717678